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II. MARCO TEÓRICO

2.2 Bases Teóricas respecto al problema 1 Ontologías

2.2.14 Base de Datos

appendix 1

Glossary

Aerobic In the presence of oxygen. Anaerobic In the absence of oxygen.

Heavy metal A term used to describe metals with a high atomic mass, some of which can be harmful to ecological and human health.

MPN Most Probable Number

Municipal Pertaining to the urban situation.

Organic micropollutants A term used to describe a huge number of compounds which are discharged into the sewerage system with wastewater from homes, industries, storm sewers, etc. Several of these have been singled out for monitoring and regulation in Biosolids on the basis of their rate of occurrence and potential hazard to human health and to the environment.

p.e. Population equivalent

1 p.e. is the organic biodegradable load having a 5-day biochemical oxygen demand of 60 g of oxygen per day. Precautionary principle A principle enshrined in Agenda 21, the declaration of

the United Nations Conference on Environment and Development (UNCED) in Rio de Janeiro, 1992, which reflects our incomplete knowledge of ecosystems. Wastewater sludge Sludge arising from the process of wastewater treatment.

appendix 2

Relevant legislation

Legislation with which this Code of Good Practice complies

Council Directive 76/464/EEC on pollution caused by certain dangerous substances discharged into the aquatic environment of the Community,

- adopted by the Local Government (Water Pollution) Act, 1977

the Local Government (Water Pollution) Amendment Act, 1990 Statutory Instrument No. 245 of 1994

Council Directive 80/68/EEC on the protection of groundwater against pollution caused by certain dangerous substances

- adopted by the Local Government (Water Pollution) Act, 1977 Statutory Instrument No. 108 of 1978

Statutory Instrument No. 390 of 1979 Statutory Instrument No. 33 of 1982

the Local Government (Water Pollution) Amendment Act, 1990 Statutory Instrument No. 245 of 1994

the Waste Management Act, 1996

Council Directive 86/278/EEC on the protection of the environment, and in particular of the soil, when sewage sludge is used in agriculture,

- adopted by Statutory Instrument No. 183 of 1991 the Waste Management Act, 1996

Council Directive 91/271/EEC concerning urban waste water treatment, - adopted by Statutory Instrument No. 419 of 1994

Council Directive 91/676/EEC concerning the protection of waters against pollution caused by nitrates from agriculture

Legislation taken into account in the preparation of this Code of

Good Practice

Council Directive 78/659/EEC on the quality of fresh waters needing protection or improvement in order to support fish life,

- adopted by the Local Government (Water Pollution) Act, 1977 Statutory Instrument No. 293 of 1988

Council Directive 83/513/EEC on cadmium discharges to the aquatic environment - adopted by Statutory Instrument No. 294 of 1985

Council Resolution 88/C 30/01 on a community action programme to combat environmental pollution by cadmium

appendix 3

Recommended treatment processes for Biosolids

production

Table 1

Recommended Treatment Process Conditions for Production of Biosolids

Process Description

Mesophilic anaerobic digestion with pre- or post- pasteurisation

Mean retention period of at least 12 days primary digestion in temperature range 35o +/- 3oC or of at least 20 days primary digestion in temperature range 25oC +/- 3oC. Pasteurisation phase must achieve a retention period of at least 1 hour at a temperature ≥ 70oC or 2 hours at a temperature ≥ 55oC.

Thermophilic anaerobic digestion Mean retention period of at least 48 – 72 hours in temperature range 50 – 55oC. Must include a retention period of at least 1 hour at a temperature greater than 70oC followed by a minimum retention period of at least 2 hours at a temperature ≥ 55oC or of at least 4 hours at a temperature ≥ 50oC.

Thermophilic aerobic digestion Mean retention period of at least 7 days. All sludge to be subject to a temperature ≥ 55oC for at least 4 hours. Must achieve a reduction in volatile solids of ≥ 38%.

Composting: 1. Windrows

2. Static pile or in-vessel

To be held at 55oC for at least 15 days, during which time a temperature of ≥ 55oC must be maintained over 5 turnings of the windrow.

A temperature of ≥ 55oC must be achieved and maintained uniformly for at least 3 days.

Alkaline stabilisation 1. Addition of lime to raise pH to greater than 12.0 with an accompanying rise in temperature to 70oC for 30 minutes.

2. Addition of lime to raise pH to greater than 12.0 and to maintain the pH above 12 for 72 hours and to achieve a temperature ≥ 52oC for at least 12 hours. At the end of the 72 hour period, air dry to a dry solid content of ≥ 50%.

Thermal drying Drying by direct or indirect contact with hot gases. Moisture content of the dried Biosolids to be ≤ 10%. Either the temperature of the Biosolids > 80oC or the wet bulb temperature of the gas in contact with the Biosolids as the Biosolids leaves the drier > 80oC.

appendix 4

Composition and fertiliser value of Biosolids

Table 1

Composition of Irish Wastewater Sludges

(Note: These are untreated sludges. Nitrogen and phosphorus composition may change with treatment. Heavy metal content will remain unchanged.)

Range Mean Number of

samples Dry solids1 % 1 – 65 22 20 Nitrogen1 mg/kgDS3 8.5 – 58100 27558 12 Phosphorus1 mg/kgDS 1.5 – 21100 10386 13 Potassium1 mg/kgDS 0.7 – 89,600 31467 3 Magnesium1 mg/kgDS – – 0.4 2 Copper1 mg/kgDS 25 – 2,481 641 24 Nickel1 mg/kgDS 2.6 – 389 54 24 Iron1 mg/kgDS 1,200 – 96,075 20,190 7 Zinc1 mg/kgDS 32 – 2070 562 25 Cadmium1 mg/kgDS 0.1 – 13.6 2.8 22 Chromium1 mg/kgDS 28 – 509 165 4 Lead1 mg/kgDS 8.1 – 850 150 24 Mercury1 mg/kgDS 0.1 – 2.0 0.6 4 Manganese2 mg/kgDS 65 – 3,018 340 N/A Boron2 mg/kg DS 19 - 236 72 N/A Cobalt2 mg/kg DS 1 – 48 14 N/A

1 Samples from 25 Irish wastewater treatment plants taken for the Strategy Study on Options for the Treatment

and Disposal of Sewage Sludge in Ireland (Weston-FTA, 1993). The smallest wastewater treatment plant in

this survey served a population of 350; the largest served a population of 29,527.

2 200 samples from 45 Irish wastewater treatment plants published in O’Riordan , E.G., Dodd, V.A., Tunney, H. and Fleming, G.A. (1986), “The chemical composition of Irish sewage sludges”. In the Irish Journal of

Agricultural Research, No. 25.

Table 2

Total and Available Phosphorus in Biosolids produced by Various Recommended Treatment Processes

Biosolids type % DS1 Total P applied Available P

(1st cropping year) Digested low-solids 4 3% of DS = 1.2 kg/tonne 60% of total P = 0.7 kg/ tonne Digested high-solids 25 3.5% of DS = 8.8 kg/tonne 35 – 50% of total P = 3.0 – 4.4 kg/tonne Composted2 65 1.0% of DS = 6.5 kg/tonne 20% of total P = 1.3 kg/tonne Lime stabilised 60 0.4% of DS = 2.4 kg/tonne 46% of total P = 1.1 kg/tonne Thermally dried 94 3.7% of DS = 34.8 kg/tonne 9 – 50% of total P = 3.1 – 17.4 kg/tonne 1 DS = dry solids

2 Wood chips used as bulking agent

Table 3

Total and Available Nitrogen in Biosolids produced by Various Recommended Treatment Processes

Biosolids type % DS1 Total N applied Available N

(1st cropping year) Digested low-solids 4 5% of DS = 2.0 kg/tonne 60% of total N = 1.2 kg/ tonne Digested high-solids 25 3.0% of DS = 7.5 kg/tonne 15% of total N = 1.1 kg/tonne Composted2 65 1.6% of DS = 10.4 kg/tonne 10% of total N3 = 1.0 kg/tonne Lime stabilised 60 0.7% of DS = 4.2 kg/tonne 15% of total N = 0.6 kg/tonne Thermally dried 94 3.7% of DS = 34.8 kg/tonne 20% of total N = 7.0 kg/tonne 1 DS = dry solids

2 Wood chips used as bulking agent 3 Ammonium-N only

appendix 5

Planting, harvesting and grazing constraints

Table 1

Planting, harvesting and grazing constraints to be observed when using Biosolids as a fertiliser

Crops to which Biosolids can be applied while growing

Crops to which Biosolids can be applied prior to sowing/setting

Cereals Oil seed rape

Grass1 Forestry2

Cereals Oil seed rape

Grass Sugar beet Animal fodder1

Forestry2 1

No harvesting or grazing until at least 3 weeks after application.

2

appendix 6

Limits to heavy metal application

Table 1

Maximum permissible concentrations of certain heavy metals in soil

Metal Maximum permissible concentration

(mg/kg dry solids) pH 5.0 – 6.0 and/or clay content 10 – 15% pH > 6.0 and clay content > 15% Zinc 100 150 Cadmium 1.0 1.5 Nickel 50 80

For pH > 5.0 and clay content 15%

Copper 80

Lead 80

Mercury 1

Chromium 100

Table 2

Maximum permissible annual average rates of addition of certain heavy metals to soils over a 10-year period

Metal Maximum permissible

average annual rate of addition of metal over a 10-year period

(kg/hectare/year) Zinc 7.5 Cadmium 0.05 Nickel 3.0 Copper 7.5 Lead 4.0 Mercury 0.1 Chromium 3.5

Table 3

Typical maximum permissible number of applications of Biosolids as determined by soil metal concentrations

Cd Cu Ni Pb Zn Cr

Case 1: Biosolids @ 2% DS; 2.8% N; 1% P

Concentration in Biosolids (mg/kg DS) 2.8 641 54 150 562 165 Background level in soil1 (mg/kg soil) 0.61 21 24.8 24.2 71.8 46.6 Amount in Biosolids

application of 50 t/ha

(kg/ha) 0.003 0.64 0.05 0.15 0.56 0.17 Total concentration in

25 cm soil sample in year 1

(mg/kg soil) 0.61 21.2 24.8 24.2 72.0 46.7 Permissible number of applications at 50 t/ha2 452 299 1516 1209 163 1051 Case 2: Biosolids @ 6% DS; 2.8% N; 1% P Concentration in Biosolids (mg/kg DS) 2.8 641 54 150 562 165 Background level in soil1 (mg/kg soil) 0.61 21 24.8 24.2 71.8 46.6 Amount in Biosolids

application of 50 t/ha

(kg/ha) 0.008 1.9 0.16 0.45 1.69 0.5 Total concentration in

25 cm soil sample in year 1

(mg/kg soil) 0.61 21.6 24.9 24.3 72.3 46.8 Permissible number of applications at 50 t/ha2 150 99 505 403 54 350 Case 3: Biosolids @ 25% DS; 2.8% N; 1% P Concentration in Biosolids (mg/kg DS) 2.8 641 54 150 562 165 Background level in soil1 (mg/kg soil) 0.61 21 24.8 24.2 71.8 46.6 Amount in Biosolids

application of 50 t/ha

(kg/ha) 0.025 5.77 0.49 1.35 5.06 1.49 Total concentration in

25 cm soil sample in year 1

(mg/kg soil) 0.62 22.8 25.0 24.6 73.6 47.1 Permissible number

of applications at 50 t/ha2

50 33 168 134 18 116

1 Average background metal concentrations in Irish agricultural soils

appendix 7

Monitoring requirements

Table 1

Parameters to be included in Certificate of Analysis of Biosolids

Parameter Units of measurement

Dry solids (%)

Organic matter (TOC as % of dry solids)

pH

Total nitrogen (% dry solids)

Ammonium-nitrogen (% dry solids)

Total phosphorus (% dry solids)

Total potassium (% dry solids)

Faecal coliform (MPN.g-1 dry solids)

Salmonella sp. (MPN.g-1 dry solids)

Zinc (mg.kg-1 dry solids)

Copper (mg.kg-1 dry solids)

Nickel (mg.kg-1 dry solids)

Cadmium (mg.kg-1 dry solids)

Lead (mg.kg-1 dry solids)

Mercury (mg.kg-1 dry solids)

Chromium (mg.kg-1 dry solids)

Polychlorinated biphenyls (PCB) (mg.kg-1 dry solids) Polychlorinated dibenzodioxins/dibenzofurans (PCDD/F) (ng TEQ.kg-1 dry solids) Polyaromatic Hydrocarbons (PAH) (mg.kg-1 dry solids)

Table 2

Minimum Frequency of Analysis of Certain Parameters required to be Monitored in Biosolids

Parameter Frequency of analysis1

< 50,000 p.e. 50,000 – 100,000 p.e. > 100,000 p.e.

pH Every 12 months2 Every 12 months Every 6 months

Total nitrogen Every 12 months2 Every 12 months Every 6 months

Ammonium-nitrogen Every 12 months2 Every 12 months Every 6 months

Total phosphorus Every 12 months2 Every 12 months Every 6 months

Total potassium Every 12 months2 Every 12 months Every 6 months

Faecal coliform Every week Every week Every week

Salmonella sp. Every week Every week Every week

Zinc Every 12 months2 Every 12 months Every 6 months

Copper Every 12 months2 Every 12 months Every 6 months

Nickel Every 12 months2 Every 12 months Every 6 months

Cadmium Every 12 months2 Every 12 months Every 6 months

Lead Every 12 months2 Every 12 months Every 6 months

Mercury Every 12 months2 Every 12 months Every 6 months

Chromium Every 12 months2 Every 12 months Every 6 months

36 Table 2 … continued

Minimum Frequency of Analysis of Certain Parameters required to be Monitored in Biosolids

Parameter Frequency of analysis1

< 50,000 p.e. 50,000 – 100,000 p.e. > 100,000 p.e.

Polychlorinated biphenyls (PCB) Every 5 years Every 2 years3 Every 12 months

Polychlorinated dibenzodioxins/dibenzofurans (PCDD/F) Every 5 years Every 2 years3 Every 12 months

Polyaromatic Hydrocarbons (PAH) Every 5 years Every 2 years3 Every 12 months

Nonylphenol Every 5 years Every 2 years3 Every 12 months

1 To be analysed more frequently if there is a significant change in the quality of the wastewater stream.

2 Can be reduced to every 2 years for a wastewater treatment plant into which industry does not discharge and if no significant changes are observed in the parameter values over a period of 2

years.

3 Can be reduced to every 5 years for a wastewater treatment plant into which industry does not discharge. Should be analysed more frequently if there is a significant change in the quality of

Table 3

Minimum Frequency of Soil Sampling and Analysis

Parameter Depth of sample

(cm)

Frequency

Organic matter 10 Every 2 years

pH 10 Every 2 years

Clay content 10 Every 2 years

Total phosphorus 10 Every 2 years

Total potassium 10 Every 2 years

Zinc 25 Every 5 years

Copper 25 Every 5 years

Nickel 25 Every 5 years

Cadmium 25 Every 5 years

Lead 25 Every 5 years

Mercury 25 Every 5 years

Chromium 25 Every 5 years

Polychlorinated biphenyls (PCB) 25 Every 5 years

Polychlorinated dibenzodioxins/dibenzofurans (PCDD/F)

25 Every 5 years

38 Table 4

Recommended Analytical Methodology to be used for Parameters to be Monitored in Biosolids

Parameter Standard Test Number1 Analytical methods

Dry solids Standard Methods 2540B Total solids dried at 103 – 105oC

Organic matter Standard Methods 5310B

BS Method

Combustion-Infrared Method Gravimetric Analysis

pH Standard Methods 4500-H+ pH metre

Total nitrogen

BS Method

Digestion with sulphuric acid and hydrogen peroxide followed by distillation

Colorimetric analysis

Ammonium-nitrogen BS Method Digestion and Colorimetric Analysis

Total phosphorus Standard Methods 4500-P Digestion and Colorimetric Analysis

Total potassium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Faecal coliform Standard Methods 9221E or 9222D Faecal Coliform Procedure: Multiple Tube or Membrane

Filter

Salmonella sp. Standard Methods 9260D Quantitative Salmonella Procedures

Zinc Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Copper Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Nickel Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method continued …

Table 4 … continued

Recommended Analytical Methodology to be used for Parameters to be Monitored in Biosolids

Parameter Standard Test Number Analytical methods

Cadmium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Standard Methods 3030D and 3113B2 Electrothermal Atomic Absorption Spectrometry

Lead Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Chromium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Mercury Standard Methods 3112 Cold Vapour Atomic Absorption

Polychlorinated biphenyls (PCB) Standard Methods 6630C Liquid-Liquid Extraction Gas Chromatography

Polychlorinated dibenzodioxins/dibenzofurans (PCDD/F)

Standard Methods 6630B Liquid-Liquid Extraction Gas Chromatography

Polyaromatic hydrocarbons (PAH) Standard Methods 6640B Liquid-Liquid Extraction Chromatography

Nonylphenol Standard Methods 5530B and C Cleanup and Chloroform Extraction

1

As specified by Standard Methods for the Examination of Water and Wastewater (American Public Health Association, American Water Works Association and Water Environment Federation), unless otherwise indicated.

2

40 Table 5

Recommended Analytical Methodology to be used for Parameters to be Monitored in Soil

Parameter Test Number1 Analytical methods

Dry solids Standard Methods 2540B Total solids dried at 103 – 105oC

pH Standard Methods 4500-H+ pH metre

Clay content BS 1377, 1990, Part 2 Hydrometer Method

Total phosphorus Standard Methods 4500-P Digestion and Colorimetric Analysis

Total potassium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Zinc Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Copper Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Nickel Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Cadmium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Standard Methods 3030D and 3113B Electrothermal Atomic Absorption Spectrometry1

Lead Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Chromium Standard Methods 3030D and 3111 or 3120B Acid Digestion and Flame Atomic Adsorption

Spectrometry or Inductively Coupled Plasma Method

Table 5 … continued

Recommended Analytical Methodology to be used for Parameters to be Monitored in Soil

Parameter Test Number1 Analytical methods

Mercury Standard Methods 3112 Cold Vapour Atomic Absorption

Polychlorinated biphenyls (PCB) Standard Methods 6630C Liquid-Liquid Extraction Gas Chromatography

Polychlorinated dibenzodioxins/dibenzofurans (PCDD/F)

Standard Methods 6630B Liquid-Liquid Extraction Gas Chromatography

Polyaromatic hydrocarbons (PAH) Standard Methods 6640B Liquid-Liquid Extraction Chromatography

1

As specified by Standard Methods for the Examination of Water and Wastewater (American Public Health Association, American Water Works Association and Water Environment Federation), unless otherwise indicated.

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