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have been developed and reviewed by Plesset and Prosperetti (1977),

Prosperetti (1984a; 1984b), Feng and Leal (1997), Brenner et al. (2002)

and Lauterborn and Kurz (2010).

Lauterborn (1976) gave a thorough investigation of the basic properties of

nonlinear oscillations of gas bubbles in liquids numerically. The response

of a bubble to a single-frequency excitation was calculated and displayed

in the form of frequency response curves, i.e., the maximum bubble radius

in steady-state oscillation (non-dimensionalized by the equilibrium bubble

radius) versus driving frequency. Figure 1.4 shows typical response curves

with special features of nonlinear oscillations. The expression n m (here,

m and n are two integers) above the peaks represents the order of the resonance. Cases with m=1 and n=2, 3… correspond to harmonics; cases withm=2, 3… andn=1 correspond to subharmonics; cases with m=2, 3… and n=2, 3… correspond to ultraharmonics. There exist thresholds for subharmonics and ultraharmonics. Figure 1.5 illustrates the threshold for

the subharmonic of the order 1 2 varying with bubble radii. For detailed

definition and the descriptions of the resonances and nonlinear phenomena

(e.g., jump phenomenon, hysteresis) mentioned above, readers are referred

Figure 1.4 Frequency response curves for a bubble in water with a radius

at rest of Rn 10 μm for different sound pressure amplitudes PA of (a) 0.4, (b) 0.5, (c) 0.6, (d) 0.7, and (e) 0.8 bar.  is the frequency of the driving sound field. 0 is the natural frequency of the bubble oscillation.

max

R is the maximum radius of the bubble during its steady-state oscillation. The numbers marked above the peaks are the orders of the

resonances, represented as n m. The dots and the arrows belong to curve (e). The arrows indicate that the corresponding stationary solution is out of

the range of the diagram or that no stationary solution could be found. In

this case the values of the amplitudes were also very high oscillating

around some value outside the diagram. This figure was adapted from Fig.

Figure 1.5 Threshold for the occurrence of the first subharmonic

oscillation (of order 1 2 at   0 2) versus the equilibrium bubble radius (solid line).  is the frequency of the driving sound field. 0 is the natural frequency of the bubble oscillation. PA is the amplitude of sound pressure. This figure was adapted from Fig. 13 of Lauterborn

(1976).

The power spectrum can be used to describe the property of bubble

oscillators. By solving the bubble motion equations, the variations of

bubble radius with time could be obtained (as shown in Figure 1.6). Then

through the Fourier transform, the “time domain” diagram could be

transformed to the “frequency domain” diagram, i.e., the power spectrum

[as shown in Figure 1.7(a)], the corresponding frequencies of the bands

resonance and its harmonics. In particular conditions, as shown in Figure

1.7(b), there are bands at  2 , 3 2 and 5 2 which represent subharmonic and ultraharmonics respectively. These lines are also typical

bands which usually appear in the scattered signals (i.e., acoustical echo of

bubble oscillations) in experiments.

Figure 1.6 Non-dimensionized bubble radius versus time. Equilibrium

bubble radius Rn is 10 μm. Sound pressure amplitude is 90 kPa. Driving

frequencyvis 207 kHz for upper diagram and 197 kHz for lower diagram. This figure was adapted from Fig. 13 of Lauterborn (1988).

Figure 1.7 Power spectrum of bubble oscillator. Equilibrium bubble radius

n

R is 10 μm. Sound pressure amplitude

207 kHz; (b) 197 kHz.

and Parlitz (1988).

Newhouse and Shanka

oscillators under a dual

1

f and f2 would contain the bands at in single-frequency

the radiated pressure at frequencies

1 2

ff . They (Newhouse and Shankar, 1984; Shanka proved that the resonance at

at f2, which means obtained through dual

(a)

(b)

1.7 Power spectrum of bubble oscillator. Equilibrium bubble radius

ound pressure amplitude is 90 kPa. Driving frequency

kHz. This figure was adapted from Fig. 13 of Lauterborn

Newhouse and Shankar (1984) pointed out that the echo of bubble

a dual-frequency acoustical excitation with frequencies

would contain the bands at f1f2 besides the typical bands frequency approach. They further gave the analytical solutions of

pressure at frequencies f1, f2 , 2f1, 2f2, f1 f2

They (Newhouse and Shankar, 1984; Shankar et al., 1986) also

the resonance at f1f2 is much sharper than the resonance , which means more accurate measurements of bubble size can be

dual-frequency approach.

1.7 Power spectrum of bubble oscillator. Equilibrium bubble radius

kPa. Driving frequencyv: (a) This figure was adapted from Fig. 13 of Lauterborn

r (1984) pointed out that the echo of bubble

with frequencies

besides the typical bands

gave the analytical solutions of

1 2

ff , and , 1986) also

the resonance

However, in multi-

bands rather than those corresponding to

driving frequencies. Fig

scattered signal of bubbles ex

frequencies f1 and

corresponding to main resonances (marked by

by □), subharmarnics (marked by

△). But besides these, there are other peaks (marked by magnitudes of which

Figure 1.8 Experimental spectr

excited by a dual-frequency ultrasound field. The frequencies of the two

sound waves are

1 2 12

ff  MHz. of Ma (2010).

-frequency systems, the scattered echo contains

those corresponding to the difference and sum

driving frequencies. Figure 1.8 is an experimental spectrum

scattered signal of bubbles excited by a dual-frequency field (with

and f2 respectively). In this figure, there are peaks corresponding to main resonances (marked by■), their harmonics (marked ), subharmarnics (marked by▲) and sum and difference (marked by

besides these, there are other peaks (marked by

of which are of the same order of the harmonics.

1.8 Experimental spectrum of the scattered signal from bubbles

frequency ultrasound field. The frequencies of the two

sound waves are f15.5 MHz and f2 6.5 MHz, respectively. 2 1 1

f  f MHz. This figure was adapted from Fig. contains more

the difference and sum of the

um of the

frequency field (with

In this figure, there are peaks

), their harmonics (marked

sum and difference (marked by

besides these, there are other peaks (marked by ◆), the

of the scattered signal from bubbles

frequency ultrasound field. The frequencies of the two

respectively.

So far as we know, most published papers mainly focused on the

application of the sum and difference of the driving frequencies in

multi-frequency systems (Wyczalkowski and Szeri, 2003; Phelps and

Leighton, 1994; Wu et al., 2005). The fundamental properties of bubble

dynamics (for instance, the special bands marked by ◆ shown in Figure 1.8) under multi-frequency acoustical excitation have not been studied

systematically. However, these features are essential for understanding the

bubble behaviour under multi-frequency excitation as well as expanding

their applications.

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