5. RESULTADOS DE LA INVESTIGACIÓN
5.2 RECOMENDACIONES
7.7
Signal to background ratio in
228Th measure-
ment
Samples of SSE events can be also collected using uncollimated228Th measurements. In the decay chain of 228Th we find 208Tl which emits the most energetic γ-line that can be found in nature with 2614.5 keV. At this energy pair production is the dom- inant process of photon interaction with matter. The positron which is created in this process materializes and subsequently annihilates with an electron emitting two photons back-to-back with an energy of 511 keV each. The photons can escape the detector in which case their energy is missing. Three characteristic lines can be see in
228Th spectra. The Full Energy Peak (FEP) of the208Tl line at 2614.5 keV, the Single
Escape Peak (SEP) at 2103.5 keV and the Double Escape Peak (DEP) at 1592.5 keV.
If both photons escape the detector the remaining energy is released in a very small volume thus events in the DEP are SSE events. The probability of both photons escaping the detector is highest on the detector surface and especially high in its corners. Hence, the spatial distribution of DEP events is very inhomogeneous.
A 228Th measurement was done with the BEGe detector at HV = 5kV with a measurement real time of about 3 h. the distribution of A/E versus the calibrated energy can be seen in Figure 7.15. The SSE events emerge as a horizontal band. To estimate the background contribution in the DEP line we fit the A/E distribution of (1592±5) keV (see Figure 7.16 with a Gaussian fit function and allow for a low energy tail (Equation 4.4). As for the 137Cs coincidence measurements, the contribution is
estimated from the two side bands left and right of the Gaussian; we find a SSE to background ratio of (11759 − 747)/747 = 14.7 ± 0.6.
Figure 7.15: A/E versus calibrated energy of a228Th measurement recorded
with the BEGe detector. The SSE events are visible as a horizontal band and the DEP with the highest SSE contribution at an energy of 1592 keV.
7.7. Signal to background ratio in 228Th measurement
The tail was not observed in the A/E distribution of the 137Cs measurement in Fig- ure 7.2 and the SSE to background ratio achieved with the 137Cs measurements is
always higher except for Run4, Run5 and Run15 (see Table 7.2). Note that these measurements were central scans and the contribution of SSE events from the de- tector center in a 228Th measurement is negligible. The best SSE to background
ratio estimated is 121.4 ± 31.7 in Run17.
Figure 7.16: 228Th A/E distribution of the DEP line. A Gaussian plus low energy tail fit is shown in red. The two side bands used to estimate the SSE to background ratio are shown as gray bands.
Chapter 8
Analysis of the background
component
42
Ar in Gerda
As already mentioned in Chapter 2 background control is essential for low back- ground experiments. All contributions have to be understood in order to minimize and estimate them. One important background component in Gerda is the β con- tinuum of42K, daughter of42Ar which is naturally present in the cryo liquid Argon
(LAr) of the Gerda setup.
8.1
Production mechanism of
42Ar
The abundance of42Ar in natural liquid Argon depends on the way42Ar is produced.
So in order to get a feeling of the order of magnitude of the specific activity of42Ar
we look for its production mechanisms.
As pointed out in [68] 42Ar can be produced via double neutron capture by 40Ar 40Ar + n −→ 41Ar + n −→ 42Ar (8.1)
They estimate the natural 42Ar abundance from both naturally occurring neutrons and neutrons which are produced in nuclear explosions and come to an estimate of 42Ar/40Ar = 7.4 · 10−22 corresponding to A(42Ar) = 7.4 µBq/kg for the latter as
dominant mechanism.
However, they do not consider the cosmic-ray production of 42Ar in the upper at-
mosphere via the reaction
40Ar + α −→ 42Ar + 2 p (8.2)
which could be about three orders of magnitude higher and therefore the main production mechanism for 42Ar [69]. The authors estimate the ratio 42Ar/40Ar
to be roughly 10−20 in the atmosphere. This would correspond to an activity of A(42Ar) ≈ 100 µBq/kg (see Appendix F). The assumptions made in both references
are more of qualitative nature though and the calculated values can only be rough estimates.
8.2. Previous measurements
8.2
Previous measurements
Before the neutrinoless double beta decay experiment Gerda was built, a pro- posal [70] was made in which an upper limit of the 42Ar specific activity in LAr of 43 µBq/kg [71] is stated (see also Appendix F). This value would suggest a lower cross section for cosmic-ray production of42Ar as assumed by [69]. Now that Gerda
has concluded Phase I data taking, this value can be checked. In fact first tests re- vealed that the background from 42Ar was a lot higher than expected from the pro-
posal and efforts were made to reduce this background by deploying Mini-Shrouds in the Gerda setup. A Mini-Shroud is a closed copper cylinder which encloses a de- tector string in order to minimize the quantity of42Ar in contact with the detectors
and to close the electric field lines.
8.3
Methodology
42Ar decays via β− decay to42K which further decays to 42Ca via another β− decay
with an endpoint of 3525.45 keV (see Figure 8.1 and Figure 8.2).
As the energy spectrum of electrons from a beta decays is continuous, this decay contributes also at lower energies to the background especially in the region of interest around Q0ν
ββ= 2039 keV.
Figure 8.1: Decay scheme of 42Ar taken from [72].
8.4. Distribution of 42K All other unstable isotopes of Argon apart from 42Ar can be neglected as source of background around Q0ν
ββ because either their lifetime is short and they have al-
ready decayed, e.g. 41Ar has a lifetime of ca. 110 min, or the endpoint energy of the
decay Qββis lower than Q0νββ, e.g. 39Ar has an endpoint energy of Qββ = 565 keV [73].
The Gerda LAr has been underground since November 2007. With the lifetime of 42Ar being ((32.9 ± 1.1) )y (measured in 1965) [74] and the lifetime of 42K being
((12.360 ± 0.01) )y, they are in secular equilibrium. This means the specific activity of 42Ar and 42K are the same.
In the following the specific activity of42Ar is calculated by estimating the activity of
42K using almost all Gerda Phase I data. We use a γ-line of the42K spectrum which
has an energy of (1524.65 ± 0.03) keV and perform a binned maximum likelihood fit using the Bayesian Analysis Toolkit (BAT) [75]. Finally the calculated specific activity is corrected for the half life of 42Ar in order to be comparable to other
measurements and theoretical values and limits.
8.4
Distribution of
42K
To estimate the specific activity of42K in the Gerda LAr we have to make assump- tions about its distribution inside the LAr and here it starts to become tricky: As
42K is born in a β− decay it is born as a positive ion namely as42K+. The detectors
are operated at high voltage (HV), typically with 4 kV inverse bias, which creates strong electric fields and under the influence of electric fields ions are drifted. With- out further measures the distribution of42K would surely be inhomogeneous.
A lot of effort was put in making most of the LAr volume as field-free as possible by deploying small, electrically grounded copper cylinders around the detectors and by shielding the HV cables. These so called Mini-Shrouds (MS) additionally form a physical barrier for 42K+ ions.
8.5
Efficiencies
The detection efficiency is a very crucial ingredient in the activity determination as it is fully anti correlated to the specific activity itself. It is determined with a Monte Carlo Simulation assuming a specific distribution of42Ar in LAr inside Gerda. The
simulation program we use is called MaGe; it is Geant4 based and is developed by the Gerda and Majorana experiments in a collaborative effort [66, 76].
8.5.1
Simulation
The Gerda setup (see Section 2) is available as MaGe [66] geometry for MC simu- lations. A cylinder of 42K decays was simulated centered on the respective detector string. It has to be large enough in order not to miss important contributions to
8.5. Efficiencies
the efficiency of the detectors. A height of 2.10 m and a radius of 1 m were chosen according to a previous study [77]. In the following we call the incident simulated particles primaries and their starting position the primary vertex.
In Figure 8.3 all primaries are plotted that deposit energy in at least one of the detectors. The simulation contains only the one string arm in the configuration starting from Run34 (see Appendix G). Decays outside the simulated volume are considered in the systematic uncertainty (see Section 8.11).
The simulated volume was split in four parts as can be seen in Figure 8.4. The top, bottom and tube volumes combined are the volume simulated outside the respective Mini-Shroud (MS). The distribution of decays inside the MS can be varied to study systematic effects on the efficiency. Afterwards, the simulations from inside the MS and those from outside the MS can be combined without re-simulating the outer part which stays the same. Also, higher statistics are achieved in this manner.
Figure 8.3: Vertex positions of primaries which deposit energy in at least one of the BEGe detectors.
Figure 8.4: LAr cylinder in which 42K decays are simulated. The cylinder
is split in four separate volumes in order to be able to simulate different distributions inside the Mini-Shroud (MS) and combine them later.
8.5. Efficiencies
In each of the above said volumes a total number of 109 decays were simulated using Decay0 [78] to create the primary vertices in order to account for correlations in γ cascade emissions. The spectrum of primary particles is plotted in Figure 8.5.
As a crosscheck of the Monte Carlo simulation a rough estimate of the branching ratio RB(1525 keV) of the 1525 keV γ-line was performed. From 1500 keV to 1550 keV
the spectrum is binned in 51 bins. Dividing in three regions of equal size we estimate the background using the side bands and subtract it from the middle region which contains the γ-line.
RB(1525 keV) = P34 i=18ni− P17 i=1ni+ P51 i=35ni Ntot = (18.071 ± 0.001) · 10−2 (8.3)
The number of entries in bin i is denoted as ni and Ntot is the total number of
simulated decays. The calculated value is in accordance with the literature value of Rlit
B(1525 keV) = (18.08 ± 0.09) · 10
−2 [72].
8.5.2
Efficiency calculation
In order to calculate the efficiency of the detectors in the Gerda setup to detect a 1525 keV γ photon from a 42K decay inside the LAr we first calculate the signal
counts in said γ-line from the output spectra of the simulations. The efficiency is then calculated as the number of signal counts divided by the total number of simulated decays. Last, the efficiencies are normalized by the simulated LAr volume and expressed as the rate per day seen for a specific activity of 1 µBq/kg.
Figure 8.5: Primary spectrum of the efficiency simulations containing 107
8.5. Efficiencies
To extract the signal counts, the energy window [1499 keV,1550 keV] of the simu- lation output spectra is subdivided in three regions of same size. B1 and B2 are
the sidebands and M denotes the middle region which contains the 42K γ-line at
≈ 1525 keV which we use to estimate the specific activity of 42Ar. Using the two
side bands we estimate the background contribution in region M and calculate the signal counts S as follows
S = M − 1
2(B1+ B2) (8.4) We calculate the efficiency ε by dividing S by the number of simulated decays Nsim
ε = S Nsim
(8.5)
To estimate the uncertainty on the efficiency we have to take the branching ratio RB
of the 1525 keV line into account. Effectively we are not calculating the efficiency on the full decay but on the 1525 keV line which we will denote as ε15
ε15=
S Nsim· RB
(8.6)
The uncertainty, which is calculated using binomial statistics, is then
∆ε15=
s
ε15(1 − ε15)
Nsim· RB
(8.7)
The uncertainty on the total efficiency ε is therefore
∆ε = s ∂ε ∂ε15 · ∆ε15 2 + ∂ε ∂RB · ∆RB 2 (8.8) ∆ε ε = s ∆ε15 ε15 2 + ∆RB RB 2 (8.9)
If we neglect the uncertainty on the branching ratio ∆RB for Nsim → ∞ this tends
to ∆ε ε ≈ ∆ε15 ε15 = s ε15(1 − ε15) Nsim· RB· ε215 = r (1 − ε15) S Nsim→∞ −→ √1 S (8.10) With RB = 0.1808 ± 0.009 [72] and ∆ε/ε ≈ 10−2 though, the uncertainty on the
branching ratio can not simply be neglected but contributes with approximately 10 % to the total uncertainty. In the following ∆ε contains this contribution. In the final analysis the efficiency enters as the rate per day which is seen by the respective detector for an 42Ar activity of 1 µBq/kg. Therefore, we define the normalized
efficiency εn as
εn = ε · mLAr· fn (8.11)
With the LAr mass mLAr given by the density of LAr ρLAr = 1.39 g/cm 3
multiplied by its volume VLAr:
8.5. Efficiencies
and the normalization factor
fn = 1 µBq kg · 8.64 · 10 4 s d = 8.64 · 10 −2 decays kg d (8.13)
Efficiencies of complementary simulations i can be combined by simply summing them up if there is no overlap of the simulated LAr volume and if they are normalized
En= Σiεn,i (8.14)
Supposing that complementary simulations are uncorrelated we add up the uncer- tainties on the single efficiencies in quadrature to obtain the combined uncertainty
Ξn =
q
Σi∆ε2n,i (8.15)
All simulations with their normalization factors are listed in Table 8.1. In order to ensure that the volume splitting, which was described in Section 8.5.1, leads to a reasonable result for the efficiencies, for detector string 3 (S3) a simulation without volume splitting as well as with volume splitting was done. S3 contains three detectors; their efficiencies for the split simulation and the full volume simulation are compared in Table 8.2.
Table 8.1: List of simulations and normalization factors. The normalization factor for inhomogeneous distributions inside the MS is the same as for the homogeneous distribution because a priori we do not know the real distribution and assume a homogeneous one.
# string position V [cm3] m [kg] m · f n 1 S1 top 2543330 3535 305.444 2 S1 bottom 2544630 3537 305.600 3 S1 tube 1500070 2085 180.152 4 S1 hom 3285.45 4.57 0.395
5 S1 near BEGe hom
6 S1 near MS hom 7 S2 all 6591250 9162 791.583 8 S3 all 6591360 9162 791.596 9 S3 top 2543320 3535 305.443 10 S3 bottom 2544630 3537 305.600 11 S3 tube 1500600 2086 180.216 12 S3 hom 2746.51 3.82 0.330
13 S3 near BEGe hom
14 S3 near MS hom
15 S4 all 6591280 9162 791.586 16 S1 AC 6591070 9162 791.561
8.5. Efficiencies
Table 8.2: Comparison of complete (all) and split efficiency simulations (hom). The split simulation has four different volume parts which are added like described in Equation 8.14. The difference ∆ = (εn(hom) −
εn(all))/εn(hom) is well within the uncertainty bounds.
hom all
name εn [10−3/d] εn [10−3/d] ∆[%]
RGI 3.75 ± 0.03 3.75 ± 0.06 -0.08 ANG4 4.27 ± 0.03 4.20 ± 0.06 1.64
RGII 3.90 ± 0.03 3.86 ± 0.06 1.01
Table 8.3: Efficiencies of all Phase I detectors with the list of simulations which were combined to calculate them. The values indicated with hom are used as central value and the nearDet and nearMS values are used to estimate a systematic uncertainty due to the inhomogeneity of 42K decays
(see Section 8.11).
hom nearDet nearMS
name εn [10−3/d] εn [10−3/d] εn [10−3/d] sim list
GD32B 1.03 ± 0.01 1.01 ± 0.01 0.94 ± 0.01 1-6 GD32C 1.10 ± 0.01 1.22 ± 0.01 1.02 ± 0.01 1-6 GD32D 1.07 ± 0.01 1.19 ± 0.01 0.98 ± 0.01 1-6 GD35B 1.20 ± 0.01 1.32 ± 0.01 1.12 ± 0.01 1-6 GD35C 0.87 ± 0.01 0.87 ± 0.01 0.80 ± 0.01 1-6 ANG3 4.23 ± 0.06 - - 15 ANG5 5.24 ± 0.07 - - 15 RGIII 4.08 ± 0.06 - - 15 RGI 3.75 ± 0.03 3.57 ± 0.03 3.59 ± 0.03 9-14 ANG4 4.27 ± 0.03 4.81 ± 0.03 4.10 ± 0.03 9-14 RGII 3.90 ± 0.03 3.97 ± 0.03 3.77 ± 0.03 9-14 GTF112 6.15 ± 0.08 - - 7 ANG2 5.43 ± 0.07 - - 7 ANG1 1.44 ± 0.03 - - 7 GTF45 5.02 ± 0.07 - - 16 GTF32 4.83 ± 0.07 - - 16