TITAN Mass Measurement of 11 Li
(and other halo nuclei)
Ryan Ringle, TRIUMF
The weather in Vancouver
(according to the tourist board)
The weather in Vancouver
(the other 364 days of the year)
Outline
ISAC @ TRIUMF
The TITAN experiment
Penning trap mass spectrometry Towards shorter half lives
Results of
11Li measurement
Results of other halo nuclei mass measurements
ISAC:
Highest power for On-Line facilities, we go up to 100µA
@ 500MeV DC proton
ISAC has 3 exper. areas:
• Low energy (60keV)
• ISAC I (cont. up 1.8 MeV/u)
• ISAC II (up to 10 MeV/
u, present license to 5 MeV/U)
Many experimental stations:
• TRINAT, Beta-NMR, 8pi, tape-station, TITAN, Co-linear laser spec, polarized beam line, etc
• DRAGON, TUDA, TACTIC, GPS (Leuven)
• TIGRESS, EMMA (2010), GPS (Maya)
ISAC at TRIUMF
Yields:
11Li - 4x104/s
74Rb - 2x104/s
62Ga - 2x103/s
The TITAN Experiment
ISAC Beam
RFQ
Cooling and Bunching
Penning Trap
Mass Measurement
EBIT
Charge State Breeding
!talk by T. Brunner"
!E ~ 20#60 keV"
Penning Trap Mass Spectrometry
3D ion confinement:
linear magnetic field +quadrupolar electric field
Resulting ion motion:
3 independent eigenmotions
!+,!-,!z
ω
c= ω
++ ω
−= q m B ω
−< ω
z< ω
+True cyclotron frequency is the sum of radial eigenmotions
Application of quadrupolar RF field causes beating between reduced cyclotron and magnetron motions
Extraction through magnetic field converts radial energy to
longitudinal energy
Measure TOF to determine the center frequency
+
R ! "c.Trf
Towards Shorter Half Lives
Measurement time scales:
initial magnetron preparation dipolar RF excitation ~ 10 ms Lorentz steerer FREE
cyclotron motion excitation (limited by half life)
R ! "c!Trf = (q/m)!B!Trf
charge breeding (increase q)
buy a bigger magnet (increase B)
different RF excitation scheme (reduce FWHM)
Ramsey excitation - S. George et al., PRL 98, 162501 (2007) Octupolar excitation - R. Ringle et al., IJMS 262, 33 (2007) S. Eliseev et al., IJMS 262, 45 (2007)
+ .
E! B!
. . .
. .
F ! = q( E ! + ! v × B ! )
net offset in ExB direction Principle: generate electric dipole
field in strong magnetic field region to move ions off axis
R. Ringle et al., IJMS 263, 38 (2007)
Penning trap benchmarks
6,7
Li mass comparison
Compare to SMILETRAP* values
*14# deviation of m(7Li) from AME03
*Sz. Nagy et al., PRL 96, 163004 (2006) Agreement is observed on the 2(7)x10-9 level
12C vs. 6Li
mass shift insignificant on the 3(4)x10-8 level over six mass units
Mass dependent frequency shifts
MTITAN-MSMILE = 13(39) eV
7Li $m/m ~ 5x10-10
Halo Nuclei
one-proton halo two-proton halo binary system
one-neutron halo two-neutron halo
four-neutron halo
measured with TITAN proposed
S 2n of All Bound Nuclei
11Li 6He
17B
14Be
27F
8He
slide from D. Lunney
Li Isotope Shifts
R. Sánchez et al., PRL 96, 033002 (2006)
altered charge radius, r
c, of
11Li could indicate a perturbed
9Li core
Isotopic Shift
mass shift term (MS)
~ 10 GHz for Li
δν
expA,A!− δν
M SA,A!= F δ < r
c2>
A,A!field shift term
~ 0.001 GHz for Li
- mass shift terms calculated by Z.-C. Yan and G.W.F. Drake
Z.-C Yan and G.W.F. Drake, PRL 91, 113004 (2003)
- 11Li mass measurement with $m " 1 keV/c2 required to remove it as a source of significant uncertainty
- 6,7Li rc determined via elastic electron scattering
- optical isotope shift measurements provide relative shift
C.W. de Jager et al., At. Data Nucl. Data Tables 14, 479 (1974)
11 Li S 2n Value
Thibault et al.Wouters et al.
Kobayashi et al.
Young et al.
Bachelet et al.
150 200 250 300 350 400
S 2n [keV]
AME '03
Five previous measurements of S
2n(
11Li)
Reference Method S2n [keV]
Thibault et al. Mass Spec. 170 ± 80 J.M. Wouters et al. TOF 320 ± 120 T. Kobayashi et al. 11B(#-,#+)11Li 340 ± 50
B.M. Young et al. 14C(11B,11Li)14O 295 ± 35 Bachelet et al. Mass Spec. 376 ± 5
AME ’03: S2n(11Li) = 300 ± 20 keV
- Need a precision of $m " 5 keV/c2 to confirm accuracy of Bachelet et al.
- An S2n(11Li) value with 1% uncertainty, $m " 3 keV/c2, would provide a solid test for nuclear theory.
PRC 12, 644 (1975)
Z. Phys. A 331, 229 (1988) KEK Rep. 91-22 (1991) PRL 71, 4124 (1993)
Eur. Phys. J. A 25, 31 (2005)
G. Audi et al., Nucl. Phys. A 729, 129 (2003)
- Need a precision of $m " 1 keV/c2 for charge radius calculations.
TITAN Mass Measurement of 9,11 Li
(preliminary)
-100 -50 0 50 100
!RF - 5147353.46 [Hz]
35 40 45 50 55 60
TOF ["s]
11Li+
#m/m ~ 7x10-8
T1/2 = 8.5 ms
-5 0 5
!RF - 6,297,542 [Hz]
37 39 41 43 45 47 49 51
TOF ["s]
9Li+
#m/m ~ 8x10-9 T1/2 = 177 ms
Measurement
-2 -1 0 1 2
M.E. TITAN - M.E. AME03 [keV]
AME03
TITAN
9Li
Measurement
-80 -60 -40 -20 0 20
M.E. TITAN-M.E. AME03 [keV]
AME03
TITAN
11Li
6 measurements
$m/m ~ 3x10-9
9 measurements
$m/m ~ 3x10-8
$m ~ 50 eV
$m ~ 550 eV
TITAN Mass Measurement of 9,11 Li
(preliminary)
-100 -50 0 50 100
!RF - 5147353.46 [Hz]
35 40 45 50 55 60
TOF ["s]
11Li+
#m/m ~ 7x10-8
T1/2 = 8.5 ms
-5 0 5
!RF - 6,297,542 [Hz]
37 39 41 43 45 47 49 51
TOF ["s]
9Li+
#m/m ~ 8x10-9 T1/2 = 177 ms
Thibault et al.Wouters et al.
Kobayashi et al.
Young et al.
Bachelet et al.
150 200 250 300 350 400
S 2n [keV]
AME '03
TITAN Mass Measurement of 9,11 Li
(preliminary)
-100 -50 0 50 100
!RF - 5147353.46 [Hz]
35 40 45 50 55 60
TOF ["s]
11Li+
#m/m ~ 7x10-8
T1/2 = 8.5 ms
-5 0 5
!RF - 6,297,542 [Hz]
37 39 41 43 45 47 49 51
TOF ["s]
9Li+
#m/m ~ 8x10-9 T1/2 = 177 ms
Thibault et al.Wouters et al.
Kobayashi et al.
Young et al.
Bachelet et al.
TITAN '07
150 200 250 300 350 400
S 2n [keV]
AME '03
(%S2n)AME03 ~ 3.5#
(%S2n)Bachelet ~ 1.4#
How Big is 8 He?
P. Mueller et al., PRL 99, 252501 (2007)
How Big is 8 He?
P. Mueller et al., PRL 99, 252501 (2007)
How Big is 8 He?
P. Mueller et al., PRL 99, 252501 (2007)
TITAN Mass Measurement of 8 He
(preliminary)
-20 -15 -10 -5 0 5 10 15 20
!rf - 7075868 [Hz]
25 30 35 40 45 50 55 60
TOF ["s]
8He+
#m/m ~ 4x10-8
Measurements
-10 -5 0 5 10 15
M.E. TITAN-M.E. AME03 [keV]
AME03 TITAN
8He
- First direct mass measurement of 8He - H2 used as buffer gas in RFQ
- $m ~ 300 eV
- Produced with “broken” FEBIAD ion source
- %m ~ 1.9#
T1/2 = 117 ms
TITAN Mass Measurement of 11 Be
(preliminary)
-5 0 5
!RF - 5,157,659 [Hz]
42 47 52 57
TOF ["s]
11Be+
#m/m ~ 1x10-8
Measurement
-8 -4 0 4 8
M.E. TITAN - AME03 [keV]
AME03
11Be
TITAN Measurements
-15 -10 -5 0 5 10 15
M.E. - AME04 [keV]
AME03
9Be(t,p)11Be
10Be(d,p)11Be
MISTRAL
TITAN
$m/m ~ 7x10-9 (reduced by a factor of ~ 50)
T1/2 = 11 s
The TITAN mass spectrometer has been commissioned and is capable of making high-precision mass measurements of very short lived nuclei
TITAN has performed precision mass measurements of He, Li and Be halo nuclei (final analysis pending).
New halo mass measurements allow a refined charge radius determination and shed new light on the structure of halo nuclei
More mass measurements to come this year (halo, CKM, structure, HCI, etc.)
Neutrinoless &&-decay measurements using EBIT (T. Brunner on Friday)
Conclusions & Outlook
The TITANs
M. Brodeur, T. Brunner, C.
Champagne, J. Dilling, P. Delheij, S. Ettenauer, M. Good, A. Lapierre, D. Lunney, R. Ringle,
V. Ryjkov, M. Smith,
and the TITAN collaboration